Mechanistic aspects of the gas-phase coupling of thioanisole and chlorobenzene to dibenzothiophene catalyzed by atomic Ho(+).

نویسندگان

  • Shaodong Zhou
  • Maria Schlangen
  • Helmut Schwarz
چکیده

Mechanistic aspects of the novel gas-phase generation of dibenzothiophene via coupling of thioanisole and chlorobenzene, employing atomic Ho(+) as a catalyst, have been investigated using Fourier-transform ion cyclotron resonance mass spectrometry in conjunction with density functional theory (DFT) calculations.

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Growth-phase dependent biodesulfurization of Dibenzothiophene by Enterobacter sp. strain NISOC-03

Petroleum-polluted soil samples from Ahvaz oilfield were enriched, using three methods to detect microorganisms with different dibenzothiophene degradation capabilities. Strain NISOC-03, a nitrate-reducing, oxidase negative, catalase, citrate, and urease positive, gram negative rod, showed interesting dibenzothiophene desulfurization behavior, designated as Entreobacter sp. strain NISOC-03 base...

متن کامل

Growth-phase dependent biodesulfurization of Dibenzothiophene by Enterobacter sp. strain NISOC-03

Petroleum-polluted soil samples from Ahvaz oilfield were enriched, using three methods to detect microorganisms with different dibenzothiophene degradation capabilities. Strain NISOC-03, a nitrate-reducing, oxidase negative, catalase, citrate, and urease positive, gram negative rod, showed interesting dibenzothiophene desulfurization behavior, designated as Entreobacter sp. strain NISOC-03 base...

متن کامل

Effects of coupling on turbulent gas-particle boundary layer flows at borderline volume fractions using kinetic theory

This study is concerned with the prediction of particles’ velocity in a dilute turbulent gas-solidboundary layer flow using a fully Eulerian two-fluid model. The closures required for equationsdescribing the particulate phase are derived from the kinetic theory of granular flows. Gas phaseturbulence is modeled by one-equation model and solid phase turbulence by MLH theory. Resultsof one-way and...

متن کامل

نمونه برداری و تعیین مقدار کلروبنزن در هوا با روش میکرواستخراج فاز جامد-گاز کروماتوگرافی طیف بین جرمی

Abstract Background and aims: The chlorobenzene is an intermediate chemical that is used in the production of commodities such as herbicides, dyestuffs, and rubber and Causes neurological complications and effects on the respiratory tract. In this research solid phase micro extraction (SPME) was used for the sampling of chlorobenzene in air. The optimum conditions for analysis with gas chrom...

متن کامل

Phase-transfer catalysis for synthesis of ethyl 2-(4-nitrophenoxy)acetate under sonication- kinetic aspects

Ultrasound assisted phase-transfer catalyzed preparation of ethyl 2-(4-nitrophenoxy)acetate from the corresponding p-nitrophenol and ethyl 2-bromoacetate using the mild solid base, anhydrous potassium carbonate, under very mild conditions is reported. The solid-liquid reactions were performed in a batch reactor equipped with reflux condenser, and ultrasonic irradiations were introduced using an...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:
  • Physical chemistry chemical physics : PCCP

دوره 17 14  شماره 

صفحات  -

تاریخ انتشار 2015